Mount Calvary United Methodist Church is located in Harlem Village, Manhattan, at 116 Edgecombe Avenue and 140th Street. The church occupies a building originally constructed for The Evangelical Lutheran Church of the Atonement in 1897, which served as a mission church. After Atonement merged with the Lutheran Church of Our Saviour, the congregation relocated. The building now serves Mount Calvary United Methodist Church, continuing its legacy as a place of worship in the community.